A study on high electrochemical capacitance of ion exchange resin-based activated carbons for supercapacitor

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Abstract

In this work, activated carbons (ACs) with high porosity are synthesized from polystyrene-based ion exchange resin (PIR) by potassium hydroxide (KOH) chemical activation, and the influence of the KOH-to-PIR ratio on the porosity of the ACs and electrochemical characteristics is investigated. As a result, PIR is successfully converted into ACs with well-developed micro and mesopores. The specific surface areas and pore volumes are increased with an increase in the KOH-to-PIR ratio. Furthermore, it is found that increasing the amount of KOH led to a transformation of the micropores into meso- and macropores. The electrochemical performance of the PIR-based ACs is enhanced by high specific surface area and oxygen functional groups. In the application to electric double-layer capacitors (EDLCs), the PIR-based AC with a KOH-to-PIR ratio of 4 (PIR-4) has the highest specific capacitance (258 F g -1) and shows excellent electrochemical stability. Thus, it is thought that the PIR-based ACs are suitable electrode materials for EDLCs.

Original languageEnglish
Pages (from-to)1039-1044
Number of pages6
JournalCurrent Applied Physics
Volume12
Issue number4
DOIs
Publication statusPublished - 1 Jul 2012
Externally publishedYes

Keywords

  • Activated carbon
  • Electric double-layer capacitor
  • Polystyrene-based ion exchangeable resin
  • Porosity

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