Application of classical models of chirality to surface second harmonic generation

F. Hache; H. Mesnil; M. C. Schanne-Klein

doi:10.1063/1.1404983

Application of classical models of chirality to surface second harmonic generation

Institut Polytechnique de Paris

Research output: Contribution to journal › Article › peer-review

Abstract

The second-order nonlinear response of an isotropic layer of chiral molecules was calculated by extending the two classical models (Kuhn and Kauzmann). Various nonlinear susceptibilities (magnetic dipolar, electric dipolar, and electric quadrupolar) were calculated. These were applied to the derivation of second harmonic field radiated by the molecules. Different results about the origin of the chiral response were obtained by the two models.

Original language	English
Pages (from-to)	6707-6715
Number of pages	9
Journal	Journal of Chemical Physics
Volume	115
Issue number	14
DOIs	https://doi.org/10.1063/1.1404983
Publication status	Published - 8 Oct 2001

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10.1063/1.1404983

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title = "Application of classical models of chirality to surface second harmonic generation",

abstract = "The second-order nonlinear response of an isotropic layer of chiral molecules was calculated by extending the two classical models (Kuhn and Kauzmann). Various nonlinear susceptibilities (magnetic dipolar, electric dipolar, and electric quadrupolar) were calculated. These were applied to the derivation of second harmonic field radiated by the molecules. Different results about the origin of the chiral response were obtained by the two models.",

author = "F. Hache and H. Mesnil and Schanne-Klein, \{M. C.\}",

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AU - Hache, F.

AU - Mesnil, H.

AU - Schanne-Klein, M. C.

PY - 2001/10/8

Y1 - 2001/10/8

N2 - The second-order nonlinear response of an isotropic layer of chiral molecules was calculated by extending the two classical models (Kuhn and Kauzmann). Various nonlinear susceptibilities (magnetic dipolar, electric dipolar, and electric quadrupolar) were calculated. These were applied to the derivation of second harmonic field radiated by the molecules. Different results about the origin of the chiral response were obtained by the two models.

AB - The second-order nonlinear response of an isotropic layer of chiral molecules was calculated by extending the two classical models (Kuhn and Kauzmann). Various nonlinear susceptibilities (magnetic dipolar, electric dipolar, and electric quadrupolar) were calculated. These were applied to the derivation of second harmonic field radiated by the molecules. Different results about the origin of the chiral response were obtained by the two models.

U2 - 10.1063/1.1404983

DO - 10.1063/1.1404983

M3 - Article

AN - SCOPUS:0035828645

SN - 0021-9606

VL - 115

SP - 6707

EP - 6715

JO - Journal of Chemical Physics

JF - Journal of Chemical Physics

IS - 14

ER -

Application of classical models of chirality to surface second harmonic generation

Abstract

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