Abstract
A recently reported variant of asynchronous optical sampling compatible with arbitrary unstabilized laser repetition rates is applied to pump-probe spectroscopy. This makes possible the use of a 5.1 MHz chirped pulse oscillator as the pump laser, thus extending the available time window to almost 200 ns with a time resolution as good as about 320 fs. The method is illustrated with the measurement in a single experiment of the complete charge transfer dynamics of the reaction center from Rhodobacter sphaeroides.
| Original language | English |
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| Pages (from-to) | 3322-3324 |
| Number of pages | 3 |
| Journal | Optics Letters |
| Volume | 38 |
| Issue number | 17 |
| DOIs | |
| Publication status | Published - 1 Sept 2013 |