Abstract
Nanoporous graphene (NPG) exhibits an apparent semiconductivity to solve the zero-gap problem of graphene and also offers multifunctionalities that are directly associated with its structural and chemical nature. However, reliable, low-cost, and large-scale production of NPG is a major challenge for its practical applications. Here, a high-performance resistive-switching memory cell based on biomass-derived NPG materials is demonstrated for the first time. A new processing method is suggested to create 3D NPG starting from Saccharum officinarum. The fabricated Au/NPG/Au two-terminal devices achieve an excellent electrical performance characterized by an operating voltage below 5 V and an ON/OFF current ratio of over 106. A range of materials and device characterizations reveal the oxygen ion migration and charge-injection modulation as a key mechanism behind the observed memory behaviors. This unconventional approach to high-performance memory devices is an important step toward sustainable electronics and intelligent technologies.
| Original language | English |
|---|---|
| Article number | 2200084 |
| Journal | Advanced Materials Interfaces |
| Volume | 9 |
| Issue number | 11 |
| DOIs | |
| Publication status | Published - 1 Apr 2022 |
Keywords
- biomass
- environmental materials
- memories
- nanoporous graphene
- resistive switching
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