Effect of side-chain length of succinic anhydride on coefficient of thermal expansion behavior of epoxy resins

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Abstract

The effect of an alkenyl side-chain of succinic anhydride (SA) on the thermal behavior and the coefficient of thermal expansion (CTE) of diglycidylether of bisphenol A (DGEBA) epoxy resins was studied. The number of carbons in the side-chain of SA was varied from 6 to 14 and N,N-Dimethylbenzylamine was used as an accelerator. As a result, the reactivity of SA with epoxide groups was decreased on increasing the length of the alkenyl side-chain of SA. The thermal stabilities of cured DGEBA/SA samples were approximately constant with varying alkenyl side-chain of SA. Also, the CTE of the systems was increased as the length of the alkenyl side-chain of SA increased. This could be attributed to the increased motion of the chain segments in the epoxy network structure induced by the longer alkenyl side-chain of SA. The effect of amount anhydride, thermoplastics, and fillers on the CTE of the epoxy resins was also discussed.

Original languageEnglish
Pages (from-to)1289-1295
Number of pages7
JournalPolymer International
Volume55
Issue number11
DOIs
Publication statusPublished - 1 Nov 2006
Externally publishedYes

Keywords

  • Crosslinking
  • Curing of polymers
  • Thermal properties
  • Thermosets

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