High-pressure chemistry of hydrocarbons relevant to planetary interiors and inertial confinement fusion

D. Kraus; N. J. Hartley; S. Frydrych; A. K. Schuster; K. Rohatsch; M. Rödel; T. E. Cowan; S. Brown; E. Cunningham; T. Van Driel; L. B. Fletcher; E. Galtier; E. J. Gamboa; A. Laso Garcia; D. O. Gericke; E. Granados; P. A. Heimann; H. J. Lee; M. J. Macdonald; A. J. Mackinnon; E. E. McBride; I. Nam; P. Neumayer; A. Pak; A. Pelka; I. Prencipe; A. Ravasio; R. Redmer; A. M. Saunders; M. Schölmerich; M. Schörner; P. Sun; S. J. Turner; A. Zettl; R. W. Falcone; S. H. Glenzer; T. Döppner; J. Vorberger

doi:10.1063/1.5017908

High-pressure chemistry of hydrocarbons relevant to planetary interiors and inertial confinement fusion

D. Kraus
, N. J. Hartley
, S. Frydrych
, A. K. Schuster
, K. Rohatsch
, M. Rödel
, T. E. Cowan
, S. Brown
, E. Cunningham
, T. Van Driel
, L. B. Fletcher
, E. Galtier
, E. J. Gamboa
, A. Laso Garcia
, D. O. Gericke
, E. Granados
, P. A. Heimann
, H. J. Lee
, M. J. Macdonald
, A. J. Mackinnon

E. E. McBride, I. Nam, P. Neumayer, A. Pak, A. Pelka, I. Prencipe, A. Ravasio, R. Redmer, A. M. Saunders, M. Schölmerich, M. Schörner, P. Sun, S. J. Turner, A. Zettl, R. W. Falcone, S. H. Glenzer, T. Döppner, J. Vorberger

Research output: Contribution to journal › Article › peer-review

Abstract

Diamond formation in polystyrene (C₈H₈)_n, which is laser-compressed and heated to conditions around 150 GPa and 5000 K, has recently been demonstrated in the laboratory [Kraus et al., Nat. Astron. 1, 606-611 (2017)]. Here, we show an extended analysis and comparison to first-principles simulations of the acquired data and their implications for planetary physics and inertial confinement fusion. Moreover, we discuss the advanced diagnostic capabilities of adding high-quality small angle X-ray scattering and spectrally resolved X-ray scattering to the platform, which shows great prospects of precisely studying the kinetics of chemical reactions in dense plasma environments at pressures exceeding 100 GPa.

Original language	English
Article number	056313
Journal	Physics of Plasmas
Volume	25
Issue number	5
DOIs	https://doi.org/10.1063/1.5017908
Publication status	Published - 1 May 2018

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Kraus, D., Hartley, N. J., Frydrych, S., Schuster, A. K., Rohatsch, K., Rödel, M., Cowan, T. E., Brown, S., Cunningham, E., Van Driel, T., Fletcher, L. B., Galtier, E., Gamboa, E. J., Laso Garcia, A., Gericke, D. O., Granados, E., Heimann, P. A., Lee, H. J., Macdonald, M. J., ... Vorberger, J. (2018). High-pressure chemistry of hydrocarbons relevant to planetary interiors and inertial confinement fusion. Physics of Plasmas, 25(5), Article 056313. https://doi.org/10.1063/1.5017908

@article{5e0fdd2dc8ad4cafa0dc6b2481d59979,

title = "High-pressure chemistry of hydrocarbons relevant to planetary interiors and inertial confinement fusion",

abstract = "Diamond formation in polystyrene (C8H8)n, which is laser-compressed and heated to conditions around 150 GPa and 5000 K, has recently been demonstrated in the laboratory [Kraus et al., Nat. Astron. 1, 606-611 (2017)]. Here, we show an extended analysis and comparison to first-principles simulations of the acquired data and their implications for planetary physics and inertial confinement fusion. Moreover, we discuss the advanced diagnostic capabilities of adding high-quality small angle X-ray scattering and spectrally resolved X-ray scattering to the platform, which shows great prospects of precisely studying the kinetics of chemical reactions in dense plasma environments at pressures exceeding 100 GPa.",

author = "D. Kraus and Hartley, \{N. J.\} and S. Frydrych and Schuster, \{A. K.\} and K. Rohatsch and M. R{\"o}del and Cowan, \{T. E.\} and S. Brown and E. Cunningham and \{Van Driel\}, T. and Fletcher, \{L. B.\} and E. Galtier and Gamboa, \{E. J.\} and \{Laso Garcia\}, A. and Gericke, \{D. O.\} and E. Granados and Heimann, \{P. A.\} and Lee, \{H. J.\} and Macdonald, \{M. J.\} and Mackinnon, \{A. J.\} and McBride, \{E. E.\} and I. Nam and P. Neumayer and A. Pak and A. Pelka and I. Prencipe and A. Ravasio and R. Redmer and Saunders, \{A. M.\} and M. Sch{\"o}lmerich and M. Sch{\"o}rner and P. Sun and Turner, \{S. J.\} and A. Zettl and Falcone, \{R. W.\} and Glenzer, \{S. H.\} and T. D{\"o}ppner and J. Vorberger",

note = "Publisher Copyright: {\textcopyright} 2018 Author(s).",

year = "2018",

month = may,

day = "1",

doi = "10.1063/1.5017908",

language = "English",

volume = "25",

journal = "Physics of Plasmas",

issn = "1070-664X",

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Kraus, D, Hartley, NJ, Frydrych, S, Schuster, AK, Rohatsch, K, Rödel, M, Cowan, TE, Brown, S, Cunningham, E, Van Driel, T, Fletcher, LB, Galtier, E, Gamboa, EJ, Laso Garcia, A, Gericke, DO, Granados, E, Heimann, PA, Lee, HJ, Macdonald, MJ, Mackinnon, AJ, McBride, EE, Nam, I, Neumayer, P, Pak, A, Pelka, A, Prencipe, I, Ravasio, A, Redmer, R, Saunders, AM, Schölmerich, M, Schörner, M, Sun, P, Turner, SJ, Zettl, A, Falcone, RW, Glenzer, SH, Döppner, T & Vorberger, J 2018, 'High-pressure chemistry of hydrocarbons relevant to planetary interiors and inertial confinement fusion', Physics of Plasmas, vol. 25, no. 5, 056313. https://doi.org/10.1063/1.5017908

TY - JOUR

T1 - High-pressure chemistry of hydrocarbons relevant to planetary interiors and inertial confinement fusion

AU - Kraus, D.

AU - Hartley, N. J.

AU - Frydrych, S.

AU - Schuster, A. K.

AU - Rohatsch, K.

AU - Rödel, M.

AU - Cowan, T. E.

AU - Brown, S.

AU - Cunningham, E.

AU - Van Driel, T.

AU - Fletcher, L. B.

AU - Galtier, E.

AU - Gamboa, E. J.

AU - Laso Garcia, A.

AU - Gericke, D. O.

AU - Granados, E.

AU - Heimann, P. A.

AU - Lee, H. J.

AU - Macdonald, M. J.

AU - Mackinnon, A. J.

AU - McBride, E. E.

AU - Nam, I.

AU - Neumayer, P.

AU - Pak, A.

AU - Pelka, A.

AU - Prencipe, I.

AU - Ravasio, A.

AU - Redmer, R.

AU - Saunders, A. M.

AU - Schölmerich, M.

AU - Schörner, M.

AU - Sun, P.

AU - Turner, S. J.

AU - Zettl, A.

AU - Falcone, R. W.

AU - Glenzer, S. H.

AU - Döppner, T.

AU - Vorberger, J.

PY - 2018/5/1

Y1 - 2018/5/1

N2 - Diamond formation in polystyrene (C8H8)n, which is laser-compressed and heated to conditions around 150 GPa and 5000 K, has recently been demonstrated in the laboratory [Kraus et al., Nat. Astron. 1, 606-611 (2017)]. Here, we show an extended analysis and comparison to first-principles simulations of the acquired data and their implications for planetary physics and inertial confinement fusion. Moreover, we discuss the advanced diagnostic capabilities of adding high-quality small angle X-ray scattering and spectrally resolved X-ray scattering to the platform, which shows great prospects of precisely studying the kinetics of chemical reactions in dense plasma environments at pressures exceeding 100 GPa.

AB - Diamond formation in polystyrene (C8H8)n, which is laser-compressed and heated to conditions around 150 GPa and 5000 K, has recently been demonstrated in the laboratory [Kraus et al., Nat. Astron. 1, 606-611 (2017)]. Here, we show an extended analysis and comparison to first-principles simulations of the acquired data and their implications for planetary physics and inertial confinement fusion. Moreover, we discuss the advanced diagnostic capabilities of adding high-quality small angle X-ray scattering and spectrally resolved X-ray scattering to the platform, which shows great prospects of precisely studying the kinetics of chemical reactions in dense plasma environments at pressures exceeding 100 GPa.

UR - https://www.scopus.com/pages/publications/85047623390

U2 - 10.1063/1.5017908

DO - 10.1063/1.5017908

M3 - Article

AN - SCOPUS:85047623390

SN - 1070-664X

VL - 25

JO - Physics of Plasmas

JF - Physics of Plasmas

IS - 5

M1 - 056313

ER -

High-pressure chemistry of hydrocarbons relevant to planetary interiors and inertial confinement fusion

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