Magnetic chiroptical effects in surface second harmonic reflection

M. C. Schanne-Klein; F. Hache; T. Brotin; C. Andraud; A. Collet

doi:10.1016/S0009-2614(01)00275-5

Magnetic chiroptical effects in surface second harmonic reflection

M. C. Schanne-Klein, F. Hache, T. Brotin, C. Andraud, A. Collet

Research output: Contribution to journal › Article › peer-review

Abstract

We perform surface second harmonic reflection (SHR) to study a chiral stilbene. It exhibits a strong circular intensity difference in the second harmonic signal, but no linear intensity difference and no rotation of polarization. This SHR optical activity is characteristic of strong magnetic effects and proves that the molecule under study exhibits a one-electron chirality.

Original language	English
Pages (from-to)	159-166
Number of pages	8
Journal	Chemical Physics Letters
Volume	338
Issue number	2-3
DOIs	https://doi.org/10.1016/S0009-2614(01)00275-5
Publication status	Published - 20 Apr 2001
Externally published	Yes

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title = "Magnetic chiroptical effects in surface second harmonic reflection",

abstract = "We perform surface second harmonic reflection (SHR) to study a chiral stilbene. It exhibits a strong circular intensity difference in the second harmonic signal, but no linear intensity difference and no rotation of polarization. This SHR optical activity is characteristic of strong magnetic effects and proves that the molecule under study exhibits a one-electron chirality.",

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year = "2001",

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doi = "10.1016/S0009-2614(01)00275-5",

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T1 - Magnetic chiroptical effects in surface second harmonic reflection

AU - Schanne-Klein, M. C.

AU - Hache, F.

AU - Brotin, T.

AU - Andraud, C.

AU - Collet, A.

PY - 2001/4/20

Y1 - 2001/4/20

N2 - We perform surface second harmonic reflection (SHR) to study a chiral stilbene. It exhibits a strong circular intensity difference in the second harmonic signal, but no linear intensity difference and no rotation of polarization. This SHR optical activity is characteristic of strong magnetic effects and proves that the molecule under study exhibits a one-electron chirality.

AB - We perform surface second harmonic reflection (SHR) to study a chiral stilbene. It exhibits a strong circular intensity difference in the second harmonic signal, but no linear intensity difference and no rotation of polarization. This SHR optical activity is characteristic of strong magnetic effects and proves that the molecule under study exhibits a one-electron chirality.

U2 - 10.1016/S0009-2614(01)00275-5

DO - 10.1016/S0009-2614(01)00275-5

M3 - Article

AN - SCOPUS:0003044059

SN - 0009-2614

VL - 338

SP - 159

EP - 166

JO - Chemical Physics Letters

JF - Chemical Physics Letters

IS - 2-3

ER -

Magnetic chiroptical effects in surface second harmonic reflection

Abstract

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