TY - JOUR
T1 - Mean age of stratospheric air derived from AirCore observations
AU - Engel, Andreas
AU - Bönisch, Harald
AU - Ullrich, Markus
AU - Sitals, Robert
AU - Membrive, Olivier
AU - Danis, Francois
AU - Crevoisier, Cyril
N1 - Publisher Copyright:
© Author(s) 2017. This work is distributed under.
PY - 2017/6/12
Y1 - 2017/6/12
N2 - Mean age of stratospheric air can be derived from observations of sufficiently long-lived trace gases with approximately linear trends in the troposphere. Mean age can serve as a tracer to investigate stratospheric transport and long-Term changes in the strength of the overturning Brewer-Dobson circulation of the stratosphere. For this purpose, a low-cost method is required in order to allow for regular observations up to altitudes of about 30ĝ€km. Despite the desired low costs, high precision and accuracy are required in order to determine mean age. We present balloon-borne AirCore observations from two midlatitude sites: Timmins in Ontario/Canada and Lindenberg in Germany. During the Timmins campaign, five AirCores sampled air in parallel with a large stratospheric balloon and were analysed for CO2, CH4 and partly CO. We show that there is good agreement between the different AirCores (better than 0.1ĝ€%), especially when vertical gradients are small. The measurements from Lindenberg were performed using small low-cost balloons and yielded very comparable results. We have used the observations to extend our long-Term data set of mean age observations at Northern Hemisphere midlatitudes. The time series now covers more than 40 years and shows a small, statistically non-significant positive trend of 0.15ĝ€±ĝ€0.18 yearsĝ€decadeĝ'1. This trend is slightly smaller than the previous estimate of 0.24ĝ€±ĝ€0.22 yearsĝ€decadeĝ'1 which was based on observations up to the year 2006. These observations are still in contrast to strong negative trends of mean age as derived from some model calculations.
AB - Mean age of stratospheric air can be derived from observations of sufficiently long-lived trace gases with approximately linear trends in the troposphere. Mean age can serve as a tracer to investigate stratospheric transport and long-Term changes in the strength of the overturning Brewer-Dobson circulation of the stratosphere. For this purpose, a low-cost method is required in order to allow for regular observations up to altitudes of about 30ĝ€km. Despite the desired low costs, high precision and accuracy are required in order to determine mean age. We present balloon-borne AirCore observations from two midlatitude sites: Timmins in Ontario/Canada and Lindenberg in Germany. During the Timmins campaign, five AirCores sampled air in parallel with a large stratospheric balloon and were analysed for CO2, CH4 and partly CO. We show that there is good agreement between the different AirCores (better than 0.1ĝ€%), especially when vertical gradients are small. The measurements from Lindenberg were performed using small low-cost balloons and yielded very comparable results. We have used the observations to extend our long-Term data set of mean age observations at Northern Hemisphere midlatitudes. The time series now covers more than 40 years and shows a small, statistically non-significant positive trend of 0.15ĝ€±ĝ€0.18 yearsĝ€decadeĝ'1. This trend is slightly smaller than the previous estimate of 0.24ĝ€±ĝ€0.22 yearsĝ€decadeĝ'1 which was based on observations up to the year 2006. These observations are still in contrast to strong negative trends of mean age as derived from some model calculations.
U2 - 10.5194/acp-17-6825-2017
DO - 10.5194/acp-17-6825-2017
M3 - Article
AN - SCOPUS:85020724457
SN - 1680-7316
VL - 17
SP - 6825
EP - 6838
JO - Atmospheric Chemistry and Physics
JF - Atmospheric Chemistry and Physics
IS - 11
ER -