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Metallicity without quasi-particles in room-temperature strontium titanate

  • Xiao Lin
  • , Carl Willem Rischau
  • , Lisa Buchauer
  • , Alexandre Jaoui
  • , Benoît Fauqué
  • , Kamran Behnia
  • PSL Research University
  • Collège de France

Research output: Contribution to journal › Article › peer-review

42 Citations (Scopus)

Abstract

Cooling oxygen-deficient strontium titanate to liquid-helium temperature leads to a decrease in its electrical resistivity by several orders of magnitude. The temperature dependence of resistivity follows a rough T3 behavior before becoming T2 in the low-temperature limit, as expected in a Fermi liquid. Here, we show that the roughly cubic resistivity above 100 K corresponds to a regime where the quasi-particle mean-free-path is shorter than the electron wave-length and the interatomic distance. These criteria define the Mott-Ioffe-Regel limit. Exceeding this limit is the hallmark of strange metallicity, which occurs in strontium titanate well below room temperature, in contrast to other perovskytes. We argue that the T3-resistivity cannot be accounted for by electron-phonon scattering à la Bloch-Gruneisen and consider an alternative scheme based on Landauer transmission between individual dopants hosting large polarons. We find a scaling relationship between carrier mobility, the electric permittivity and the frequency of transverse optical soft mode in this temperature range. Providing an account of this observation emerges as a challenge to theory.

Original languageEnglish
Article number44
Journalnpj Quantum Materials
Volume2
Issue number1
DOIs
Publication statusPublished - 1 Dec 2017
Externally publishedYes

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