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Multiphoton k -resolved photoemission from gold surface states with 800-nm femtosecond laser pulses

  • Fausto Sirotti
  • , Nathan Beaulieu
  • , Azzedine Bendounan
  • , Mathieu G. Silly
  • , Christian Chauvet
  • , Gregory Malinowski
  • , Guido Fratesi
  • , Valérie Véniard
  • , Giovanni Onida
  • Synchrotron SOLEIL
  • Université Paris-Saclay
  • Dipartimento di Fisica
  • University of Milano
  • CNISM and Dipartimento di Scienza Dei Materiali
  • University of Milano-Bicocca
  • European Theoretical Spectroscopy Facility (ETSF

Research output: Contribution to journalArticlepeer-review

23 Citations (Scopus)

Abstract

We measure direct multiphoton photoemission of the Au(111) surface state with 800-nm laser pulses. We observe the parabolic dispersion in the angular distribution of photoelectrons having absorbed between four and seven photons. The k≥ dispersion we measure can be explained in terms of Shockley-state replicas, with a nascent hot electrons distribution at k≥ above the Fermi level. Moderate laser power densities, of the order of 100GW/cm2, resulted in large electron yields, indicating the importance of multiphoton excitations to define the electronic and magnetic properties of matter in the first hundred femtoseconds after laser excitation.

Original languageEnglish
Article number035401
JournalPhysical Review B - Condensed Matter and Materials Physics
Volume90
Issue number3
DOIs
Publication statusPublished - 2 Jul 2014

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