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Nano-plasmonic near field phase matching of attosecond pulses

  • Tahir Shaaran
  • , Rana Nicolas
  • , Bianca Iwan
  • , Milutin Kovacev
  • , Hamed Merdji
  • Université Paris-Saclay
  • Leibniz Universität Hannover, Institut für Quantenoptik
  • Centre for Quantum Engineering and Space-Time Research
  • QUEST Institute for Experimental Quantum Metrology

Research output: Contribution to journal › Article › peer-review

14 Citations (Scopus)

Abstract

Nano-structures excited by light can enhance locally the electric field when tuned to plasmonic resonances. This phenomenon can be used to boost non-linear processes such as harmonic generation in crystals or in gases, Raman excitation, and four wave mixing. Here we present a theoretical investigation of the near-field phase matching of attosecond pulses emitted by high-order harmonic generation (HHG) of an atom immersed in a multi-cycle femtosecond infrared laser field and a spatially inhomogeneous plasmonic field. We demonstrate that the spatial inhomogeneity factor of the plasmonic field strongly affects the electron trajectory and recombination time which can be used to control the attosecond emission. For further insight into the plasmonic field effect, we monitor the phase of each quantum path as a function of the inhomogeneity strength. Moreover, we investigate the attosecond emission as a function of near-field phase matching effects. This is achieved by calculating the coherent field superposition of attosecond pulses emitted from various intensities or field inhomogeneities. Finally, far-field and near-field phase matching effects are combined to modulate the harmonic spectral phase towards the emission of a single attosecond pulse.

Original languageEnglish
Article number6356
JournalScientific Reports
Volume7
Issue number1
DOIs
Publication statusPublished - 1 Dec 2017
Externally publishedYes

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