Nonlinear THz Control of Lead Halide Perovskite Lattices in 3, 2, and 1 Dimensions

Joanna M. Urban; Maximilian Frenzel; Marie Cherasse; Gaelle Trippe-Allard; Abdelaziz Jouaiti; Sylvie Ferlay; Emmanuelle Deleporte; Sebastian F. Maehrlein

doi:10.1109/IRMMW-THz57677.2023.10299222

Nonlinear THz Control of Lead Halide Perovskite Lattices in 3, 2, and 1 Dimensions

Joanna M. Urban
, Maximilian Frenzel
, Marie Cherasse
, Gaelle Trippe-Allard
, Abdelaziz Jouaiti
, Sylvie Ferlay
, Emmanuelle Deleporte
, Sebastian F. Maehrlein

Research output: Chapter in Book/Report/Conference proceeding › Conference contribution › peer-review

Abstract

Lead halide perovskites (LHPs) have emerged as promising semiconductor materials for next-generation optoelectronic devices such as solar cells or LEDs. The origin of their surprising optoelectronic properties have been linked to a delicate interplay of their complex lattice structure and electronic degrees of freedom. Here, we demonstrate coherent THz control of lead halide's octahedral twist modes, being highly relevant for structural phase fluctuations and dynamic disorder. We discuss the different nonlinear driving mechanisms and give an outlook for lattice control of dimensionality-tailored LHPs in three, two, and one dimensions.

Original language	English
Title of host publication	IRMMW-THz 2023 - 48th Conference on Infrared, Millimeter, and Terahertz Waves
Publisher	IEEE Computer Society
ISBN (Electronic)	9798350336603
DOIs	https://doi.org/10.1109/IRMMW-THz57677.2023.10299222
Publication status	Published - 1 Jan 2023
Event	48th International Conference on Infrared, Millimeter, and Terahertz Waves, IRMMW-THz 2023 - Montreal, Canada Duration: 17 Sept 2023 → 22 Sept 2023

Publication series

Name	International Conference on Infrared, Millimeter, and Terahertz Waves, IRMMW-THz
ISSN (Print)	2162-2027
ISSN (Electronic)	2162-2035

Conference

Conference	48th International Conference on Infrared, Millimeter, and Terahertz Waves, IRMMW-THz 2023
Country/Territory	Canada
City	Montreal
Period	17/09/23 → 22/09/23

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10.1109/IRMMW-THz57677.2023.10299222

Cite this

Urban, J. M., Frenzel, M., Cherasse, M., Trippe-Allard, G., Jouaiti, A., Ferlay, S., Deleporte, E., & Maehrlein, S. F. (2023). Nonlinear THz Control of Lead Halide Perovskite Lattices in 3, 2, and 1 Dimensions. In IRMMW-THz 2023 - 48th Conference on Infrared, Millimeter, and Terahertz Waves (International Conference on Infrared, Millimeter, and Terahertz Waves, IRMMW-THz). IEEE Computer Society. https://doi.org/10.1109/IRMMW-THz57677.2023.10299222

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title = "Nonlinear THz Control of Lead Halide Perovskite Lattices in 3, 2, and 1 Dimensions",

abstract = "Lead halide perovskites (LHPs) have emerged as promising semiconductor materials for next-generation optoelectronic devices such as solar cells or LEDs. The origin of their surprising optoelectronic properties have been linked to a delicate interplay of their complex lattice structure and electronic degrees of freedom. Here, we demonstrate coherent THz control of lead halide's octahedral twist modes, being highly relevant for structural phase fluctuations and dynamic disorder. We discuss the different nonlinear driving mechanisms and give an outlook for lattice control of dimensionality-tailored LHPs in three, two, and one dimensions.",

author = "Urban, \{Joanna M.\} and Maximilian Frenzel and Marie Cherasse and Gaelle Trippe-Allard and Abdelaziz Jouaiti and Sylvie Ferlay and Emmanuelle Deleporte and Maehrlein, \{Sebastian F.\}",

note = "Publisher Copyright: {\textcopyright} 2023 IEEE.; 48th International Conference on Infrared, Millimeter, and Terahertz Waves, IRMMW-THz 2023 ; Conference date: 17-09-2023 Through 22-09-2023",

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doi = "10.1109/IRMMW-THz57677.2023.10299222",

language = "English",

series = "International Conference on Infrared, Millimeter, and Terahertz Waves, IRMMW-THz",

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Urban, JM, Frenzel, M, Cherasse, M, Trippe-Allard, G, Jouaiti, A, Ferlay, S, Deleporte, E & Maehrlein, SF 2023, Nonlinear THz Control of Lead Halide Perovskite Lattices in 3, 2, and 1 Dimensions. in IRMMW-THz 2023 - 48th Conference on Infrared, Millimeter, and Terahertz Waves. International Conference on Infrared, Millimeter, and Terahertz Waves, IRMMW-THz, IEEE Computer Society, 48th International Conference on Infrared, Millimeter, and Terahertz Waves, IRMMW-THz 2023, Montreal, Canada, 17/09/23. https://doi.org/10.1109/IRMMW-THz57677.2023.10299222

Nonlinear THz Control of Lead Halide Perovskite Lattices in 3, 2, and 1 Dimensions. / Urban, Joanna M.; Frenzel, Maximilian; Cherasse, Marie et al.
IRMMW-THz 2023 - 48th Conference on Infrared, Millimeter, and Terahertz Waves. IEEE Computer Society, 2023. (International Conference on Infrared, Millimeter, and Terahertz Waves, IRMMW-THz).

Research output: Chapter in Book/Report/Conference proceeding › Conference contribution › peer-review

TY - GEN

T1 - Nonlinear THz Control of Lead Halide Perovskite Lattices in 3, 2, and 1 Dimensions

AU - Urban, Joanna M.

AU - Frenzel, Maximilian

AU - Cherasse, Marie

AU - Trippe-Allard, Gaelle

AU - Jouaiti, Abdelaziz

AU - Ferlay, Sylvie

AU - Deleporte, Emmanuelle

AU - Maehrlein, Sebastian F.

PY - 2023/1/1

Y1 - 2023/1/1

N2 - Lead halide perovskites (LHPs) have emerged as promising semiconductor materials for next-generation optoelectronic devices such as solar cells or LEDs. The origin of their surprising optoelectronic properties have been linked to a delicate interplay of their complex lattice structure and electronic degrees of freedom. Here, we demonstrate coherent THz control of lead halide's octahedral twist modes, being highly relevant for structural phase fluctuations and dynamic disorder. We discuss the different nonlinear driving mechanisms and give an outlook for lattice control of dimensionality-tailored LHPs in three, two, and one dimensions.

AB - Lead halide perovskites (LHPs) have emerged as promising semiconductor materials for next-generation optoelectronic devices such as solar cells or LEDs. The origin of their surprising optoelectronic properties have been linked to a delicate interplay of their complex lattice structure and electronic degrees of freedom. Here, we demonstrate coherent THz control of lead halide's octahedral twist modes, being highly relevant for structural phase fluctuations and dynamic disorder. We discuss the different nonlinear driving mechanisms and give an outlook for lattice control of dimensionality-tailored LHPs in three, two, and one dimensions.

UR - https://www.scopus.com/pages/publications/85177697855

U2 - 10.1109/IRMMW-THz57677.2023.10299222

DO - 10.1109/IRMMW-THz57677.2023.10299222

M3 - Conference contribution

AN - SCOPUS:85177697855

T3 - International Conference on Infrared, Millimeter, and Terahertz Waves, IRMMW-THz

BT - IRMMW-THz 2023 - 48th Conference on Infrared, Millimeter, and Terahertz Waves

PB - IEEE Computer Society

T2 - 48th International Conference on Infrared, Millimeter, and Terahertz Waves, IRMMW-THz 2023

Y2 - 17 September 2023 through 22 September 2023

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Urban JM, Frenzel M, Cherasse M, Trippe-Allard G, Jouaiti A, Ferlay S et al. Nonlinear THz Control of Lead Halide Perovskite Lattices in 3, 2, and 1 Dimensions. In IRMMW-THz 2023 - 48th Conference on Infrared, Millimeter, and Terahertz Waves. IEEE Computer Society. 2023. (International Conference on Infrared, Millimeter, and Terahertz Waves, IRMMW-THz). doi: 10.1109/IRMMW-THz57677.2023.10299222

Nonlinear THz Control of Lead Halide Perovskite Lattices in 3, 2, and 1 Dimensions

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