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Quantitative disentanglement of coherent and incoherent laser-induced surface deformations by time-resolved x-ray reflectivity

  • M. Sander
  • , J. E. Pudell
  • , M. Herzog
  • , M. Bargheer
  • , R. Bauer
  • , V. Besse
  • , V. Temnov
  • , P. Gaal
  • University of Potsdam
  • Helmholtz-Zentrum Berlin für Materialien und Energie GmbH
  • Universität Hamburg
  • Le Mans Universite

Research output: Contribution to journalArticlepeer-review

Abstract

We present time-resolved x-ray reflectivity measurements on laser excited coherent and incoherent surface deformations of thin metallic films. Based on a kinematical diffraction model, we derive the surface amplitude from the diffracted x-ray intensity and resolve transient surface excursions with sub-Å spatial precision and 70 ps temporal resolution. The analysis allows for decomposition of the surface amplitude into multiple coherent acoustic modes and a substantial contribution from incoherent phonons which constitute the sample heating.

Original languageEnglish
Article number261903
JournalApplied Physics Letters
Volume111
Issue number26
DOIs
Publication statusPublished - 25 Dec 2017
Externally publishedYes

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