Quantum-classical model for the surface plasmon enhanced photoemission process at metal surfaces

The main purpose of this work is to propose a theoretical description of the surface plasmon polariton stimulated electron emission process at metal surfaces in which the primary electron ejection from the conduction band is treated quantum mechanically in order to go beyond the approximate approaches used up to now to represent this first step. Our theoretical results are well supported by experimental energy spectra obtained for some tens of femtosecond laser pulses impinging on a gold grating target at various intensities in the GW/cm2 range. The present model which allows us to discuss various features of the surface plasmon photoemission process such as the role of the surface plasmon phase is rather simple and could be applied with slight modifications to study the stimulated photoemission of metallic nanoparticles which has been a subject of growing interest during the past few years.