Time resolved luminescence of solids excited by femtosecond VUV pulses and synchrotron radiation

M. Kirm; V. Babin; E. Feldbach; V. Nagirnyi; S. Vielhauer; S. Guizard; B. Carré; M. D. De Grazia; H. Merdji; A. N. Belsky; N. Fedorov; P. Martin

doi:10.1002/pssc.200673876

Time resolved luminescence of solids excited by femtosecond VUV pulses and synchrotron radiation

M. Kirm
, V. Babin
, E. Feldbach
, V. Nagirnyi
, S. Vielhauer
, S. Guizard
, B. Carré
, M. D. De Grazia
, H. Merdji
, A. N. Belsky
, N. Fedorov
, P. Martin

University Tartu
Laboratoire des Solides Irradiés
CEA/UVSQ/CNRS
CELIA, Université Bordeaux i, UMR 5107 (CNRS, Bordeaux 1, CEA)

Research output: Contribution to journal › Conference article › peer-review

9 Citations (Scopus)

Abstract

Time-resolved luminescence spectroscopy has been widely used in studies of electronic excitations and their dynamics in insulators. Present paper discusses the potential of vacuum ultraviolet spectroscopy applied for wide band gap crystals using classical synchrotron radiation as well as more recently developed pulsed femtosecond short-wavelength light sources. Optical spectroscopy using novel free electron lasers and laser systems based on higher harmonic generation process allow detailed investigation of the interaction between electronic excitations and behaviour of solids under extreme radiation conditions. Significant changes in the quantum yield and emission decay kinetics as well as surface damage of single crystals were observed for CdWO₄ and CaWO₄ crystals studied in the temperature range of 8-300 K. However, in the range of excitation densities applied, up to ∼10 ¹² W/cm², the nature of luminescence centres and their characteristic emission spectra remained similar to those observed at low excitation densities.

Original language	English
Pages (from-to)	870-876
Number of pages	7
Journal	Physica Status Solidi (C) Current Topics in Solid State Physics
Volume	4
Issue number	3
DOIs	https://doi.org/10.1002/pssc.200673876
Publication status	Published - 1 Jan 2007
Externally published	Yes
Event	10th Europhysical Conference on Defects in Insulating Materials, EURODIM 2006 - Milano, Italy Duration: 10 Jul 2006 → 14 Jul 2006

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10.1002/pssc.200673876

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Kirm, M., Babin, V., Feldbach, E., Nagirnyi, V., Vielhauer, S., Guizard, S., Carré, B., De Grazia, M. D., Merdji, H., Belsky, A. N., Fedorov, N., & Martin, P. (2007). Time resolved luminescence of solids excited by femtosecond VUV pulses and synchrotron radiation. Physica Status Solidi (C) Current Topics in Solid State Physics, 4(3), 870-876. https://doi.org/10.1002/pssc.200673876

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title = "Time resolved luminescence of solids excited by femtosecond VUV pulses and synchrotron radiation",

abstract = "Time-resolved luminescence spectroscopy has been widely used in studies of electronic excitations and their dynamics in insulators. Present paper discusses the potential of vacuum ultraviolet spectroscopy applied for wide band gap crystals using classical synchrotron radiation as well as more recently developed pulsed femtosecond short-wavelength light sources. Optical spectroscopy using novel free electron lasers and laser systems based on higher harmonic generation process allow detailed investigation of the interaction between electronic excitations and behaviour of solids under extreme radiation conditions. Significant changes in the quantum yield and emission decay kinetics as well as surface damage of single crystals were observed for CdWO4 and CaWO4 crystals studied in the temperature range of 8-300 K. However, in the range of excitation densities applied, up to ∼10 12 W/cm2, the nature of luminescence centres and their characteristic emission spectra remained similar to those observed at low excitation densities.",

author = "M. Kirm and V. Babin and E. Feldbach and V. Nagirnyi and S. Vielhauer and S. Guizard and B. Carr{\'e} and \{De Grazia\}, \{M. D.\} and H. Merdji and Belsky, \{A. N.\} and N. Fedorov and P. Martin",

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doi = "10.1002/pssc.200673876",

language = "English",

volume = "4",

pages = "870--876",

journal = "Physica Status Solidi (C) Current Topics in Solid State Physics",

issn = "1862-6351",

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note = "10th Europhysical Conference on Defects in Insulating Materials, EURODIM 2006 ; Conference date: 10-07-2006 Through 14-07-2006",

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Kirm, M, Babin, V, Feldbach, E, Nagirnyi, V, Vielhauer, S, Guizard, S, Carré, B, De Grazia, MD, Merdji, H, Belsky, AN, Fedorov, N & Martin, P 2007, 'Time resolved luminescence of solids excited by femtosecond VUV pulses and synchrotron radiation', Physica Status Solidi (C) Current Topics in Solid State Physics, vol. 4, no. 3, pp. 870-876. https://doi.org/10.1002/pssc.200673876

TY - JOUR

T1 - Time resolved luminescence of solids excited by femtosecond VUV pulses and synchrotron radiation

AU - Kirm, M.

AU - Babin, V.

AU - Feldbach, E.

AU - Nagirnyi, V.

AU - Vielhauer, S.

AU - Guizard, S.

AU - Carré, B.

AU - De Grazia, M. D.

AU - Merdji, H.

AU - Belsky, A. N.

AU - Fedorov, N.

AU - Martin, P.

PY - 2007/1/1

Y1 - 2007/1/1

N2 - Time-resolved luminescence spectroscopy has been widely used in studies of electronic excitations and their dynamics in insulators. Present paper discusses the potential of vacuum ultraviolet spectroscopy applied for wide band gap crystals using classical synchrotron radiation as well as more recently developed pulsed femtosecond short-wavelength light sources. Optical spectroscopy using novel free electron lasers and laser systems based on higher harmonic generation process allow detailed investigation of the interaction between electronic excitations and behaviour of solids under extreme radiation conditions. Significant changes in the quantum yield and emission decay kinetics as well as surface damage of single crystals were observed for CdWO4 and CaWO4 crystals studied in the temperature range of 8-300 K. However, in the range of excitation densities applied, up to ∼10 12 W/cm2, the nature of luminescence centres and their characteristic emission spectra remained similar to those observed at low excitation densities.

AB - Time-resolved luminescence spectroscopy has been widely used in studies of electronic excitations and their dynamics in insulators. Present paper discusses the potential of vacuum ultraviolet spectroscopy applied for wide band gap crystals using classical synchrotron radiation as well as more recently developed pulsed femtosecond short-wavelength light sources. Optical spectroscopy using novel free electron lasers and laser systems based on higher harmonic generation process allow detailed investigation of the interaction between electronic excitations and behaviour of solids under extreme radiation conditions. Significant changes in the quantum yield and emission decay kinetics as well as surface damage of single crystals were observed for CdWO4 and CaWO4 crystals studied in the temperature range of 8-300 K. However, in the range of excitation densities applied, up to ∼10 12 W/cm2, the nature of luminescence centres and their characteristic emission spectra remained similar to those observed at low excitation densities.

U2 - 10.1002/pssc.200673876

DO - 10.1002/pssc.200673876

M3 - Conference article

AN - SCOPUS:36049029225

SN - 1862-6351

VL - 4

SP - 870

EP - 876

JO - Physica Status Solidi (C) Current Topics in Solid State Physics

JF - Physica Status Solidi (C) Current Topics in Solid State Physics

IS - 3

T2 - 10th Europhysical Conference on Defects in Insulating Materials, EURODIM 2006

Y2 - 10 July 2006 through 14 July 2006

ER -

Time resolved luminescence of solids excited by femtosecond VUV pulses and synchrotron radiation

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