Towards efficient terbium-based solution-processed OLEDs: Hole mobility increase by the ligand design

Makarii I. Kozlov; Andrey N. Aslandukov; Andrey A. Vashchenko; Aleksei V. Medved'ko; Alexey E. Aleksandrov; Egor V. Latipov; Alexander S. Goloveshkin; Dmitri A. Lypenko; Alexey R. Tameev; Valentina V. Utochnikova

doi:10.1016/j.jallcom.2021.161319

Towards efficient terbium-based solution-processed OLEDs: Hole mobility increase by the ligand design

Makarii I. Kozlov, Andrey N. Aslandukov, Andrey A. Vashchenko, Aleksei V. Medved'ko, Alexey E. Aleksandrov, Egor V. Latipov, Alexander S. Goloveshkin, Dmitri A. Lypenko, Alexey R. Tameev, Valentina V. Utochnikova

Research output: Contribution to journal › Article › peer-review

Abstract

The approach towards the increase of the terbium electroluminescence efficiency by the increase of the transport properties was further developed. Therefore, terbium-based emitters, containing anionic ligands, able to both increase the hole mobility and to sensitize terbium luminescence, were purposefully obtained within the composite films, containing the recently studied host material PO4, able to increase electron-transport properties and also to ensure terbium luminescence. As a result, the luminance of 332 cd/m² was reached, which is one of the highest results for solution-processed OLEDs based on terbium complexes.

Original language	English
Article number	161319
Journal	Journal of Alloys and Compounds
Volume	887
DOIs	https://doi.org/10.1016/j.jallcom.2021.161319
Publication status	Published - 20 Dec 2021
Externally published	Yes

Keywords

Aromatic carboxylates
Charge carrier mobility
Luminescence
Rare earth compounds
Solution-processed OLED
Thin films

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10.1016/j.jallcom.2021.161319

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Kozlov, M. I., Aslandukov, A. N., Vashchenko, A. A., Medved'ko, A. V., Aleksandrov, A. E., Latipov, E. V., Goloveshkin, A. S., Lypenko, D. A., Tameev, A. R., & Utochnikova, V. V. (2021). Towards efficient terbium-based solution-processed OLEDs: Hole mobility increase by the ligand design. Journal of Alloys and Compounds, 887, Article 161319. https://doi.org/10.1016/j.jallcom.2021.161319

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title = "Towards efficient terbium-based solution-processed OLEDs: Hole mobility increase by the ligand design",

abstract = "The approach towards the increase of the terbium electroluminescence efficiency by the increase of the transport properties was further developed. Therefore, terbium-based emitters, containing anionic ligands, able to both increase the hole mobility and to sensitize terbium luminescence, were purposefully obtained within the composite films, containing the recently studied host material PO4, able to increase electron-transport properties and also to ensure terbium luminescence. As a result, the luminance of 332 cd/m2 was reached, which is one of the highest results for solution-processed OLEDs based on terbium complexes.",

keywords = "Aromatic carboxylates, Charge carrier mobility, Luminescence, Rare earth compounds, Solution-processed OLED, Thin films",

author = "Kozlov, \{Makarii I.\} and Aslandukov, \{Andrey N.\} and Vashchenko, \{Andrey A.\} and Medved'ko, \{Aleksei V.\} and Aleksandrov, \{Alexey E.\} and Latipov, \{Egor V.\} and Goloveshkin, \{Alexander S.\} and Lypenko, \{Dmitri A.\} and Tameev, \{Alexey R.\} and Utochnikova, \{Valentina V.\}",

note = "Publisher Copyright: {\textcopyright} 2021 Elsevier B.V.",

year = "2021",

month = dec,

day = "20",

doi = "10.1016/j.jallcom.2021.161319",

language = "English",

volume = "887",

journal = "Journal of Alloys and Compounds",

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TY - JOUR

T1 - Towards efficient terbium-based solution-processed OLEDs

T2 - Hole mobility increase by the ligand design

AU - Kozlov, Makarii I.

AU - Aslandukov, Andrey N.

AU - Vashchenko, Andrey A.

AU - Medved'ko, Aleksei V.

AU - Aleksandrov, Alexey E.

AU - Latipov, Egor V.

AU - Goloveshkin, Alexander S.

AU - Lypenko, Dmitri A.

AU - Tameev, Alexey R.

AU - Utochnikova, Valentina V.

PY - 2021/12/20

Y1 - 2021/12/20

N2 - The approach towards the increase of the terbium electroluminescence efficiency by the increase of the transport properties was further developed. Therefore, terbium-based emitters, containing anionic ligands, able to both increase the hole mobility and to sensitize terbium luminescence, were purposefully obtained within the composite films, containing the recently studied host material PO4, able to increase electron-transport properties and also to ensure terbium luminescence. As a result, the luminance of 332 cd/m2 was reached, which is one of the highest results for solution-processed OLEDs based on terbium complexes.

AB - The approach towards the increase of the terbium electroluminescence efficiency by the increase of the transport properties was further developed. Therefore, terbium-based emitters, containing anionic ligands, able to both increase the hole mobility and to sensitize terbium luminescence, were purposefully obtained within the composite films, containing the recently studied host material PO4, able to increase electron-transport properties and also to ensure terbium luminescence. As a result, the luminance of 332 cd/m2 was reached, which is one of the highest results for solution-processed OLEDs based on terbium complexes.

KW - Aromatic carboxylates

KW - Charge carrier mobility

KW - Luminescence

KW - Rare earth compounds

KW - Solution-processed OLED

KW - Thin films

UR - https://www.scopus.com/pages/publications/85111906138

U2 - 10.1016/j.jallcom.2021.161319

DO - 10.1016/j.jallcom.2021.161319

M3 - Article

AN - SCOPUS:85111906138

SN - 0925-8388

VL - 887

JO - Journal of Alloys and Compounds

JF - Journal of Alloys and Compounds

M1 - 161319

ER -

Towards efficient terbium-based solution-processed OLEDs: Hole mobility increase by the ligand design

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Keywords

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