CO2-CH4 conversion and syngas formation at atmospheric pressure using a multi-electrode dielectric barrier discharge

A. Ozkan; T. Dufour; G. Arnoult; P. De Keyzer; A. Bogaerts; F. Reniers

doi:10.1016/j.jcou.2015.01.002

CO₂-CH₄ conversion and syngas formation at atmospheric pressure using a multi-electrode dielectric barrier discharge

A. Ozkan
, T. Dufour
, G. Arnoult
, P. De Keyzer
, A. Bogaerts
, F. Reniers

Chimie Analytique et Chimie des Interfaces
Université Libre de Bruxelles
Research Group PLASMANT
University of Antwerp

Résultats de recherche: Contribution à un journal › Article › Revue par des pairs

117 Citations (Scopus)

Résumé

The conversion of CO₂ and CH₄ into value-added chemicals is studied in a new geometry of a dielectric barrier discharge (DBD) with multi-electrodes, dedicated to the treatment of high gas flow rates. Gas chromatography is used to define the CO₂ and CH₄ conversion as well as the yields of the products of decomposition (CO, O₂ and H₂) and of recombination (C₂H₄, C₂H₆ and CH₂O). The influence of three parameters is investigated on the conversion: the CO₂ and CH₄ flow rates, the plasma power and the nature of the carrier gas (argon or helium). The energy efficiency of the CO₂ conversion is estimated and compared with those of similar atmospheric plasma sources. Our DBD reactor shows a good compromise between a good energy efficiency and the treatment of a large CO₂ flow rate.

langue originale	Anglais
Pages (de - à)	74-81
Nombre de pages	8
journal	Journal of CO2 Utilization
Volume	9
Les DOIs	https://doi.org/10.1016/j.jcou.2015.01.002
état	Publié - 1 janv. 2015
Modification externe	Oui

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10.1016/j.jcou.2015.01.002

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title = "CO2-CH4 conversion and syngas formation at atmospheric pressure using a multi-electrode dielectric barrier discharge",

abstract = "The conversion of CO2 and CH4 into value-added chemicals is studied in a new geometry of a dielectric barrier discharge (DBD) with multi-electrodes, dedicated to the treatment of high gas flow rates. Gas chromatography is used to define the CO2 and CH4 conversion as well as the yields of the products of decomposition (CO, O2 and H2) and of recombination (C2H4, C2H6 and CH2O). The influence of three parameters is investigated on the conversion: the CO2 and CH4 flow rates, the plasma power and the nature of the carrier gas (argon or helium). The energy efficiency of the CO2 conversion is estimated and compared with those of similar atmospheric plasma sources. Our DBD reactor shows a good compromise between a good energy efficiency and the treatment of a large CO2 flow rate.",

keywords = "Atmospheric plasma, CO conversion, DBD plasma source, Energy efficiency, Syngas production",

author = "A. Ozkan and T. Dufour and G. Arnoult and \{De Keyzer\}, P. and A. Bogaerts and F. Reniers",

year = "2015",

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T1 - CO2-CH4 conversion and syngas formation at atmospheric pressure using a multi-electrode dielectric barrier discharge

AU - Ozkan, A.

AU - Dufour, T.

AU - Arnoult, G.

AU - De Keyzer, P.

AU - Bogaerts, A.

AU - Reniers, F.

PY - 2015/1/1

Y1 - 2015/1/1

N2 - The conversion of CO2 and CH4 into value-added chemicals is studied in a new geometry of a dielectric barrier discharge (DBD) with multi-electrodes, dedicated to the treatment of high gas flow rates. Gas chromatography is used to define the CO2 and CH4 conversion as well as the yields of the products of decomposition (CO, O2 and H2) and of recombination (C2H4, C2H6 and CH2O). The influence of three parameters is investigated on the conversion: the CO2 and CH4 flow rates, the plasma power and the nature of the carrier gas (argon or helium). The energy efficiency of the CO2 conversion is estimated and compared with those of similar atmospheric plasma sources. Our DBD reactor shows a good compromise between a good energy efficiency and the treatment of a large CO2 flow rate.

AB - The conversion of CO2 and CH4 into value-added chemicals is studied in a new geometry of a dielectric barrier discharge (DBD) with multi-electrodes, dedicated to the treatment of high gas flow rates. Gas chromatography is used to define the CO2 and CH4 conversion as well as the yields of the products of decomposition (CO, O2 and H2) and of recombination (C2H4, C2H6 and CH2O). The influence of three parameters is investigated on the conversion: the CO2 and CH4 flow rates, the plasma power and the nature of the carrier gas (argon or helium). The energy efficiency of the CO2 conversion is estimated and compared with those of similar atmospheric plasma sources. Our DBD reactor shows a good compromise between a good energy efficiency and the treatment of a large CO2 flow rate.

KW - Atmospheric plasma

KW - CO conversion

KW - DBD plasma source

KW - Energy efficiency

KW - Syngas production

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DO - 10.1016/j.jcou.2015.01.002

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