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Mean age of stratospheric air derived from AirCore observations

  • Andreas Engel
  • , Harald Bönisch
  • , Markus Ullrich
  • , Robert Sitals
  • , Olivier Membrive
  • , Francois Danis
  • , Cyril Crevoisier
  • Goethe University Frankfurt am Main
  • Institute of Meteorology and Climate Research
  • Université Paris-Saclay

Résultats de recherche: Contribution à un journalArticleRevue par des pairs

Résumé

Mean age of stratospheric air can be derived from observations of sufficiently long-lived trace gases with approximately linear trends in the troposphere. Mean age can serve as a tracer to investigate stratospheric transport and long-Term changes in the strength of the overturning Brewer-Dobson circulation of the stratosphere. For this purpose, a low-cost method is required in order to allow for regular observations up to altitudes of about 30ĝ€km. Despite the desired low costs, high precision and accuracy are required in order to determine mean age. We present balloon-borne AirCore observations from two midlatitude sites: Timmins in Ontario/Canada and Lindenberg in Germany. During the Timmins campaign, five AirCores sampled air in parallel with a large stratospheric balloon and were analysed for CO2, CH4 and partly CO. We show that there is good agreement between the different AirCores (better than 0.1ĝ€%), especially when vertical gradients are small. The measurements from Lindenberg were performed using small low-cost balloons and yielded very comparable results. We have used the observations to extend our long-Term data set of mean age observations at Northern Hemisphere midlatitudes. The time series now covers more than 40 years and shows a small, statistically non-significant positive trend of 0.15ĝ€±ĝ€0.18 yearsĝ€decadeĝ'1. This trend is slightly smaller than the previous estimate of 0.24ĝ€±ĝ€0.22 yearsĝ€decadeĝ'1 which was based on observations up to the year 2006. These observations are still in contrast to strong negative trends of mean age as derived from some model calculations.

langue originaleAnglais
Pages (de - à)6825-6838
Nombre de pages14
journalAtmospheric Chemistry and Physics
Volume17
Numéro de publication11
Les DOIs
étatPublié - 12 juin 2017
Modification externeOui

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