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Mn local moments prevent superconductivity in iron pnictides Ba(Fe 1xMn x) 2As 2

  • Y. Texier
  • , Y. Laplace
  • , P. Mendels
  • , J. T. Park
  • , G. Friemel
  • , D. L. Sun
  • , D. S. Inosov
  • , C. T. Lin
  • , J. Bobroff
  • Laboratoire de Physique des Solides
  • Institut Universitaire de France
  • CNRS

Résultats de recherche: Contribution à un journalArticleRevue par des pairs

48 Citations (Scopus)

Résumé

75As nuclear magnetic resonance (NMR) experiments were performed on Ba(Fe 1xMn x) 2As 2 (x Mn=2.5%, 5% and 12%) single crystals. The Fe layer magnetic susceptibility far from Mn atoms is probed by the 75As NMR line shift and is found similar to that of BaFe 2As 2, implying that Mn does not induce charge doping. A satellite line associated with the Mn nearest neighbours (n.n.) of 75As displays a Curie-Weiss shift which demonstrates that Mn carries a local magnetic moment. This is confirmed by the main line broadening typical of a RKKY-like Mn-induced staggered spin polarization. The Mn moment is due to the localization of the additional Mn hole. These findings explain why Mn does not induce superconductivity in the pnictides contrary to other dopants such as Co, Ni, Ru or K.

langue originaleAnglais
Numéro d'article17002
journalEPL
Volume99
Numéro de publication1
Les DOIs
étatPublié - 1 juil. 2012
Modification externeOui

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