Résumé
The signature of optical activity in the third order nonlinear response of an isotropic liquid of chiral molecules is examined. A general calculation is performed to determine the existence of a nonlinear circular dichroism. Using simple classical calculations based on anharmonic oscillators in the Kuhn or Kauzmann models, the impact of the origin of the optical activity on a pump/probe study is determined. The study is carried out on a Ruthenium-tris(bipyridyl) salt with a 1 kHz femtosecond optical parametric amplifier operating at 470 nm and the polarization is modulated by a Pockels cell.
| langue originale | Anglais |
|---|---|
| Pages | 165 |
| Nombre de pages | 1 |
| état | Publié - 1 janv. 2000 |
| Evénement | 2000 International Quantum Electronics Conference (IQEC 2000) - Nice, France Durée: 10 sept. 2000 → 15 sept. 2000 |
Une conférence
| Une conférence | 2000 International Quantum Electronics Conference (IQEC 2000) |
|---|---|
| La ville | Nice, France |
| période | 10/09/00 → 15/09/00 |
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