Realization of a Density-Dependent Peierls Phase in a Synthetic, Spin-Orbit Coupled Rydberg System

We experimentally realize a Peierls phase in the hopping amplitude of excitations carried by Rydberg atoms, and observe the resulting characteristic chiral motion in a minimal setup of three sites. Our demonstration relies on the intrinsic spin-orbit coupling of the dipolar exchange interaction combined with time-reversal symmetry breaking by a homogeneous external magnetic field. Remarkably, the phase of the hopping amplitude between two sites strongly depends on the occupancy of the third site, thus leading to a correlated hopping associated with a density-dependent Peierls phase. We experimentally observe this density-dependent hopping and show that the excitations behave as anyonic particles with a nontrivial phase under exchange. Finally, we confirm the dependence of the Peierls phase on the geometrical arrangement of the Rydberg atoms.