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Shock-driven amorphization and melting in Fe2O3

  • Céline Crépisson
  • , Alexis Amouretti
  • , Marion Harmand
  • , Chrystèle Sanloup
  • , Patrick Heighway
  • , Sam Azadi
  • , David McGonegle
  • , Thomas Campbell
  • , Juan Pintor
  • , David Alexander Chin
  • , Ethan Smith
  • , Linda Hansen
  • , Alessandro Forte
  • , Thomas Gawne
  • , Hae Ja Lee
  • , Bob Nagler
  • , Yuanfeng Shi
  • , Guillaume Fiquet
  • , François Guyot
  • , Mikako Makita
  • Alessandra Benuzzi-Mounaix, Tommaso Vinci, Kohei Miyanishi, Norimasa Ozaki, Tatiana Pikuz, Hirotaka Nakamura, Keiichi Sueda, Toshinori Yabuuchi, Makina Yabashi, Justin S. Wark, Danae N. Polsin, Sam M. Vinko

Résultats de recherche: Contribution à un journalArticleRevue par des pairs

Résumé

We present measurements on Fe2O3 amorphization and melt under laser-driven shock compression up to 209(10) GPa via time-resolved in situ x-ray diffraction. At 122(3) GPa, a diffuse signal is observed indicating the presence of a noncrystalline phase. Structure factors have been extracted up to 182(6) GPa showing the presence of two well-defined peaks. A rapid change in the intensity ratio of the two peaks is identified between 145(12) and 151(12) GPa, indicative of a phase change. The noncrystalline diffuse scattering is consistent with shock amorphization of Fe2O3 between 122(3) and 145(12) GPa, followed by an amorphous-to-liquid transition above 151(12) GPa. Upon release, a noncrystalline phase is observed alongside crystalline α-Fe2O3. The extracted structure factor and pair distribution function of this release phase resemble those reported for Fe2O3 melt at ambient pressure.

langue originaleAnglais
Numéro d'article024209
journalPhysical Review B
Volume111
Numéro de publication2
Les DOIs
étatPublié - 1 janv. 2025
Modification externeOui

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