Theoretical investigation of the nonlinear circular dichroism in a liquid of chiral molecules

F. Hache; M. C. Schanne-Klein; H. Mesnil

Theoretical investigation of the nonlinear circular dichroism in a liquid of chiral molecules

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Résumé

Introducing nonlocal effects such as magnetic dipolar and electric quadrupolar ones in the time-dependent perturbation theory, we analyze the signature of optical activity in the nonlinear response of a liquid of chiral molecules. In particular, we show that such a liquid should display a nonlinear circular dichroism. Expressions for a three-level system are given.

langue originale	Anglais
Pages (de - à)	153-158
Nombre de pages	6
journal	Molecular Crystals and Liquid Crystals Science and Technology Section B: Nonlinear Optics
Volume	25
Numéro de publication	1-4
état	Publié - 1 déc. 2000

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title = "Theoretical investigation of the nonlinear circular dichroism in a liquid of chiral molecules",

abstract = "Introducing nonlocal effects such as magnetic dipolar and electric quadrupolar ones in the time-dependent perturbation theory, we analyze the signature of optical activity in the nonlinear response of a liquid of chiral molecules. In particular, we show that such a liquid should display a nonlinear circular dichroism. Expressions for a three-level system are given.",

keywords = "Chiral molecules, Nonlinear optics, Optical activity",

author = "F. Hache and Schanne-Klein, \{M. C.\} and H. Mesnil",

year = "2000",

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language = "English",

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pages = "153--158",

journal = "Molecular Crystals and Liquid Crystals Science and Technology Section B: Nonlinear Optics",

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T1 - Theoretical investigation of the nonlinear circular dichroism in a liquid of chiral molecules

AU - Hache, F.

AU - Schanne-Klein, M. C.

AU - Mesnil, H.

PY - 2000/12/1

Y1 - 2000/12/1

N2 - Introducing nonlocal effects such as magnetic dipolar and electric quadrupolar ones in the time-dependent perturbation theory, we analyze the signature of optical activity in the nonlinear response of a liquid of chiral molecules. In particular, we show that such a liquid should display a nonlinear circular dichroism. Expressions for a three-level system are given.

AB - Introducing nonlocal effects such as magnetic dipolar and electric quadrupolar ones in the time-dependent perturbation theory, we analyze the signature of optical activity in the nonlinear response of a liquid of chiral molecules. In particular, we show that such a liquid should display a nonlinear circular dichroism. Expressions for a three-level system are given.

KW - Chiral molecules

KW - Nonlinear optics

KW - Optical activity

M3 - Article

AN - SCOPUS:0034454737

SN - 1058-7268

VL - 25

SP - 153

EP - 158

JO - Molecular Crystals and Liquid Crystals Science and Technology Section B: Nonlinear Optics

JF - Molecular Crystals and Liquid Crystals Science and Technology Section B: Nonlinear Optics

IS - 1-4

ER -

Theoretical investigation of the nonlinear circular dichroism in a liquid of chiral molecules

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